Answer
1 mol of $Cl_2$ has the greater number of atoms.
Work Step by Step
1 mol of $Cl$:
1 mol of $Cl$ = 1 mol of atoms.
1 mol of $Cl_2$:
1 $Cl_2$ molecule has 2 $Cl$ atoms; therefore, 1 mol of $Cl_2$ has 2 moles of $Cl$ atoms.
2 moles of atoms > 1 mol of atoms.
1 mol $Cl_2$ > 1 mol $Cl$